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Preparation of high efficient photoelectrode of N–F-codoped TiO2 nanotubes

Paper ID Volume ID Publish Year Pages File Format Full-Text
29154 44127 2008 9 PDF Available
Title
Preparation of high efficient photoelectrode of N–F-codoped TiO2 nanotubes
Abstract

In order to obtain TiO2 electrode with high photoelectrocatalytic activity, a novel N–F-codoped TiO2 nanotubes electrode was prepared by electrochemical anodization of Ti in C2H2O4·2H2O + NH4F electrolyte. The prepared electrode had a highly self-organized structure with high-specific surface area, and N and F were successfully doped into the lattice of TiO2. When voltage during anodization was 20 V, annealing temperature was 673 K and anodic bias potential in the photoelectrocatalytic degradation was 0.25 V, N–F-codoped TiO2 nanotubes electrode showed the higher catalytic activity. In addition, there was an obvious synergetic effect between the electrochemical and photocatalytic processes, and the synergetic factor R reached 8.7. This high-synergetic effect was attributed to the advantages of photoelectrocatalytic technique using high-aspect-ratio TiO2 nanotubes and the promoting effect of N–F-codoping on the catalytic activity. Moreover, N–F-codoped TiO2 nanotubes electrode showed good stability and after five times the photoelectrocatalytic efficiencies of MO still kept above 97% within 80 min.

Keywords
TiO2 nanotubes electrode; N–F-codoping; Anodization; Photoelectrocatalysis
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Preparation of high efficient photoelectrode of N–F-codoped TiO2 nanotubes
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Publisher
Database: Elsevier - ScienceDirect
Journal: Journal of Photochemistry and Photobiology A: Chemistry - Volume 194, Issues 2–3, 20 February 2008, Pages 152–160
Authors
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Subjects
Physical Sciences and Engineering Chemical Engineering Bioengineering
Get Full-Text Now
Don't Miss Today's Special Offer
Price was $35.95
You save - $31
Price after discount Only $4.95
100% Money Back Guarantee
Full-text PDF Download
Online Support
Any Questions? feel free to contact us