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Charge-transfer as a mechanism for controlling molecular fragmentation

Paper ID Volume ID Publish Year Pages File Format Full-Text
29193 44130 2006 5 PDF Available
Title
Charge-transfer as a mechanism for controlling molecular fragmentation
Abstract

We investigate control over molecular fragmentation in the halogen substituted acetone 1,1-dibromo-3,3,3-trifluoroacetone using shaped ultrafast laser pulses. Following insight gained from closed-loop learning control experiments, further tests reveal that control over the CF3+/CHBr2+ ratio exploits a charge-transfer mechanism. We interpret the control in terms of adiabatic rapid passage.

Keywords
Coherent control; Charge-transfer; Ultrafast spectroscopy; Wave packet dynamics
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Publisher
Database: Elsevier - ScienceDirect
Journal: Journal of Photochemistry and Photobiology A: Chemistry - Volume 180, Issue 3, 25 June 2006, Pages 277–281
Authors
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Subjects
Physical Sciences and Engineering Chemical Engineering Bioengineering
Get Full-Text Now
Don't Miss Today's Special Offer
Price was $35.95
You save - $31
Price after discount Only $4.95
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Full-text PDF Download
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