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Iron oxide functionalised MIL-101 materials in aqueous phase selective oxidations

Paper ID Volume ID Publish Year Pages File Format Full-Text
40371 45851 2013 6 PDF Available
Title
Iron oxide functionalised MIL-101 materials in aqueous phase selective oxidations
Abstract

A highly active Fe containing MIL-101 material has been prepared by using a simple microwave-assisted deposition methodology. The material, characterized by several techniques including N2 physisorption, XPS and TEM, was found to have a significantly enhanced acidity due to the incorporation of ca. 2 wt.% Fe in the form of hematite Fe2O3 phase. Fe/MIL-101 exhibited excelling activities in aqueous phase oxidations of alcohols and alkenes using hydrogen peroxide as green oxidant.

Graphical abstractFigure optionsDownload full-size imageDownload high-quality image (125 K)Download as PowerPoint slideHighlights► Fe/MIL-101 was synthesized by a microwave methodology. ► Lewis acidity in materials was remarkably enhanced upon Fe incorporation. ► Fe/MIL-101 exhibited excelling activities in oxidations using hydrogen peroxide.

Keywords
Heterogeneous catalysis; Metal-organic frameworks; Microwave chemistry; Nanoparticles; Oxidation
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Publisher
Database: Elsevier - ScienceDirect
Journal: Applied Catalysis A: General - Volume 455, 30 March 2013, Pages 261–266
Authors
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Subjects
Physical Sciences and Engineering Chemical Engineering Catalysis
Get Full-Text Now
Don't Miss Today's Special Offer
Price was $35.95
You save - $31
Price after discount Only $4.95
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