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An efficient bifunctional catalyst of TiO2 coating and supported Pd on cordierite for one-pot synthesis of MIBK from acetone

Paper ID Volume ID Publish Year Pages File Format Full-Text
49299 46733 2015 4 PDF Available
Title
An efficient bifunctional catalyst of TiO2 coating and supported Pd on cordierite for one-pot synthesis of MIBK from acetone
Abstract

•A novel bifunctional catalyst for MIBK synthesis was proposed.•It exhibited 75% MIBK selectivity and 60% acetone conversion.•A high stability of bifunctional catalyst was observed.

We report here an efficient bifunctional catalyst of TiO2 coating and supported Pd on cordierite (T500/Cor&Pd/Cor) for one-pot synthesis of MIBK from acetone. The obtained 75% MIBK selectivity at 60% acetone conversion was the best performance ever reported for metal oxide based catalyst, without obvious deactivation for at least 12 h on stream. The superior performance of T500/Cor&Pd/Cor could be attributed to the dominant base sites and moderate acid sites on TiO2 coating caused by the nanoscale anatase crystallite, and its combination style of being physically mixed with Pd.

Keywords
Methyl isobutyl ketone; One-pot synthesis; TiO2 coating; Bifunctional catalysis
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An efficient bifunctional catalyst of TiO2 coating and supported Pd on cordierite for one-pot synthesis of MIBK from acetone
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Publisher
Database: Elsevier - ScienceDirect
Journal: Catalysis Communications - Volume 71, 5 November 2015, Pages 61–64
Authors
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Subjects
Physical Sciences and Engineering Chemical Engineering Catalysis
Get Full-Text Now
Don't Miss Today's Special Offer
Price was $35.95
You save - $31
Price after discount Only $4.95
100% Money Back Guarantee
Full-text PDF Download
Online Support
Any Questions? feel free to contact us