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Effective Baeyer–Villiger oxidation of ketones over germanosilicates

Paper ID Volume ID Publish Year Pages File Format Full-Text
49503 46750 2014 4 PDF Available
Title
Effective Baeyer–Villiger oxidation of ketones over germanosilicates
Abstract

•Germanosilicates efficiently catalyze the Baeyer–Villiger oxidation of ketones.•Germanosilicates are active for both 2-admantanone and cyclohexanone.•Ge-related Lewis acid sites are assumed to be the active sites.•Germanosilicates show a good stability during Baeyer–Villiger oxidation.

Germanosilicates with various topologies (UTL, BEC, UWY, IWR) serve as efficient heterogeneous catalysts for the Baeyer–Villiger oxidation of ketones. The tetrahedrally coordinated Ge ions in germanosilicates exhibited Lewis acidity, and acted as the active sites for converting ketones to corresponding lactones effectively.

Keywords
Germanosilicates; Zeolites; Heterogeneous catalysis; Baeyer–Villiger oxidation
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Effective Baeyer–Villiger oxidation of ketones over germanosilicates
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Publisher
Database: Elsevier - ScienceDirect
Journal: Catalysis Communications - Volume 55, 5 October 2014, Pages 83–86
Authors
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Subjects
Physical Sciences and Engineering Chemical Engineering Catalysis
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