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Understanding on the origins of hydroxyapatite stabilized gold nanoparticles as high-efficiency catalysts for formaldehyde and benzene oxidation

Paper ID Volume ID Publish Year Pages File Format Full-Text
49546 46751 2015 6 PDF Available
Title
Understanding on the origins of hydroxyapatite stabilized gold nanoparticles as high-efficiency catalysts for formaldehyde and benzene oxidation
Abstract

•Phosphate groups interacted and stabilized nano-gold at lower temperature.•Hydroxyl group contributed to the stabilization at higher temperature.•Au/HAP is highly active and stable for HCHO oxidation at room temperature.

Hydroxyapatite as a green and abundant material was found to enhance the stabilization of gold nanoparticles against sintering. The origins of such stabilization of HAP on supported gold nanoparticles were investigated in the present study. Phosphate groups interacted and stabilized nano-gold at lower temperature (≤ 400 °C), while hydroxyl group contributed to the stabilization at higher temperature (≤ 600 °C). Both of them contributed to the strong sintering-resistant for calcination as high as 600 °C. For the first time we found that Au/HAP and Au/CeO2/HAP catalysts are highly active and stable for formaldehyde and benzene oxidation.

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Keywords
Hydroxyapatite; Sintering-resistance; Supported gold catalysts; VOC oxidation; Cerium oxide
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Publisher
Database: Elsevier - ScienceDirect
Journal: Catalysis Communications - Volume 59, 10 January 2015, Pages 195–200
Authors
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Subjects
Physical Sciences and Engineering Chemical Engineering Catalysis
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