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Thermo-responsive polymer micelle-based nanoreactors for intelligent polyoxometalate catalysis

Paper ID Volume ID Publish Year Pages File Format Full-Text
49924 46773 2015 5 PDF Available
Title
Thermo-responsive polymer micelle-based nanoreactors for intelligent polyoxometalate catalysis
Abstract

•Thermo-responsive polymer micelle-based nanoreactor was fabricated.•It contained polyoxometalates and poly(N-isopropylacrylamide)-block-poly(L-lysine).•The wet hydrogen peroxide oxidation of phenol was chosen as a catalysis model.•The catalytic activity could be controlled.

A series of polymer micelle-based nanoreactor containing polyoxometalates and poly(N-isopropylacrylamide)-block-poly(L-lysine) (PNIPAM-b-PLys-POM) have been successfully constructed. By adjusting the molar ratio of NIPAM/Lys, the temperature-depend catalytic activity of PNIPAM-b-PLys-POM towards catalytic wet hydrogen peroxide oxidation can be controlled. This work highlights the potential of using thermo-responsive micelles as a platform for developing smart catalyst system.

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Keywords
Thermo-responsive; Polyoxometalates; Smart catalysts
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Thermo-responsive polymer micelle-based nanoreactors for intelligent polyoxometalate catalysis
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Publisher
Database: Elsevier - ScienceDirect
Journal: Catalysis Communications - Volume 58, 5 January 2015, Pages 164–168
Authors
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Subjects
Physical Sciences and Engineering Chemical Engineering Catalysis
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