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Transfer hydrogenation of methyl levulinate into gamma-valerolactone, 1,4-pentanediol, and 1-pentanol over Cu–ZrO2 catalyst under solvothermal conditions

Paper ID Volume ID Publish Year Pages File Format Full-Text
49947 46774 2016 4 PDF Available
Title
Transfer hydrogenation of methyl levulinate into gamma-valerolactone, 1,4-pentanediol, and 1-pentanol over Cu–ZrO2 catalyst under solvothermal conditions
Abstract

•A simple solvothermal method was introduced into the sequential conversion of methyl levulinate (ML).•Various yields of diverse products were obtained by tuning a series of factors.•Catalyst 2.5-CZ-550 showed a better performance because of its rich acid content and Cu0 species on the surface.

Diverse products were obtained from transfer hydrogenation of methyl levulinate (ML) by adjusting different factors under solvothermal conditions. Excellent yields of gamma-valerolactone (GVL, 75%), 1,4-pentanediol (1,4-PDO, 39%), and 1-pentanol (1-PAO, 13.8%) could be obtained using zirconium-supported copper catalyst calcined at 550 °C and under optimal conditions.

Graphical abstractRelatively mild and operational solvothermal conditions were used for hydrogenation of ML to GVL, 1,4-PDO, and 1-PAO over zirconium-supported copper catalysts.Figure optionsDownload full-size imageDownload as PowerPoint slide

Keywords
Solvothermal conditions; Isopropanol; Copper–zirconium catalysts; Methyl levulinate; Transfer hydrogenation
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Transfer hydrogenation of methyl levulinate into gamma-valerolactone, 1,4-pentanediol, and 1-pentanol over Cu–ZrO2 catalyst under solvothermal conditions
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Publisher
Database: Elsevier - ScienceDirect
Journal: Catalysis Communications - Volume 76, 10 February 2016, Pages 50–53
Authors
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Subjects
Physical Sciences and Engineering Chemical Engineering Catalysis
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Price was $35.95
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Price after discount Only $4.95
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