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Postsynthetic modification of metal–organic framework as a highly efficient and recyclable catalyst for three-component (aldehyde–alkyne–amine) coupling reaction

Paper ID Volume ID Publish Year Pages File Format Full-Text
49969 46775 2012 5 PDF Available
Title
Postsynthetic modification of metal–organic framework as a highly efficient and recyclable catalyst for three-component (aldehyde–alkyne–amine) coupling reaction
Abstract

A MOF-supported Cu(I) catalyst bearing N,O-chelating ligand was prepared through postsynthetic modification of IRMOF-3 and used as an efficient heterogeneous catalyst for three-component coupling reaction of aldehyde, alkyne, and amine. The catalyst exhibited both high catalytic activity and stability for the reaction and the framework of Cu(I) catalyst was mainly maintained after the catalyst was reused for four times.

Graphical abstractPostsynthetic modification of metal–organic framework as a highly efficient and recyclable catalyst for three-component (aldehyde–alkyne–amine) coupling reaction.Figure optionsDownload full-size imageDownload as PowerPoint slideHighlights► A Cu(I) complex was immobilized to IRMOF-3 via postsynthetic modification. ► The MOF-supported Cu(I) catalyst was used for the A3-coupling reaction. ► The Cu(I) catalyst exhibited good activity and structural stability.

Keywords
Cu(I)–MOF catalyst; Metal–organic framework; Postsynthetic modification; Heterogeneous catalyst
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Postsynthetic modification of metal–organic framework as a highly efficient and recyclable catalyst for three-component (aldehyde–alkyne–amine) coupling reaction
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Publisher
Database: Elsevier - ScienceDirect
Journal: Catalysis Communications - Volume 27, 5 October 2012, Pages 58–62
Authors
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Subjects
Physical Sciences and Engineering Chemical Engineering Catalysis
Get Full-Text Now
Don't Miss Today's Special Offer
Price was $35.95
You save - $31
Price after discount Only $4.95
100% Money Back Guarantee
Full-text PDF Download
Online Support
Any Questions? feel free to contact us