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Fine-tuning the local structure and catalytic activity of titanium-amine functionalized silica in oxidation of limonene by aqueous hydrogen peroxide

Paper ID Volume ID Publish Year Pages File Format Full-Text
50786 46813 2012 4 PDF Available
Title
Fine-tuning the local structure and catalytic activity of titanium-amine functionalized silica in oxidation of limonene by aqueous hydrogen peroxide
Abstract

Titanium-amine functionalized silica was successfully prepared by a so-called one-pot approach by using 3-aminopropyltrimethoxysilane (APTMS), tetraethoxysilane (TEOS) and titanium(IV) sulfate as precursors. It is demonstrated that the TEOS/APTMS molar ratio in the synthesis of titanium-amine functionalized silica affected the local coordination of titanium and its corresponding positive impact on catalytic activity in oxidation of limonene by aqueous hydrogen peroxide.

Graphical abstractFigure optionsDownload full-size imageDownload as PowerPoint slideHighlights► Titanium-amine functionalized silica is synthesized by one-pot approach. ► The fine-tuning local structure titanium-amine functionalized silica. ► The local coordination of titanium affected by TEOS/APTMS molar ratio. ► The local structure of titanium affects catalytic activity in oxidation of limonene.

Keywords
Local coordination of titanium; Titanium-amine functionalized silica; Limonene oxidation
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Fine-tuning the local structure and catalytic activity of titanium-amine functionalized silica in oxidation of limonene by aqueous hydrogen peroxide
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Publisher
Database: Elsevier - ScienceDirect
Journal: Catalysis Communications - Volume 20, 5 April 2012, Pages 85–88
Authors
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Subjects
Physical Sciences and Engineering Chemical Engineering Catalysis
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Don't Miss Today's Special Offer
Price was $35.95
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Price after discount Only $4.95
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Full-text PDF Download
Online Support
Any Questions? feel free to contact us