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Investigation of the effect of total pressure on performance of the catalytic water–gas shift reaction using simulated coal-derived syngases

Paper ID Volume ID Publish Year Pages File Format Full-Text
51182 46834 2009 4 PDF Available
Title
Investigation of the effect of total pressure on performance of the catalytic water–gas shift reaction using simulated coal-derived syngases
Abstract

The effect of operating pressure on the water–gas shift (WGS) reaction rate over an iron-based high-temperature catalyst, and a Co–Mo based sour-shift catalyst, was investigated using simulated coal-derived syngas at 450 °C. For both catalysts, it was found that the CO conversion rate depends linearly upon total operating pressure. The apparent reaction orders used in a power-law rate expression, where the reaction orders were derived from experimental results at atmospheric pressure, are valid at elevated pressures up to at least 11 bar.

Keywords
Water–gas shift reaction; Fe–Cr oxide catalyst; Sour-shift catalyst; Kinetics; Effect of pressure
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Investigation of the effect of total pressure on performance of the catalytic water–gas shift reaction using simulated coal-derived syngases
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Publisher
Database: Elsevier - ScienceDirect
Journal: Catalysis Communications - Volume 11, Issue 4, 15 December 2009, Pages 272–275
Authors
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Subjects
Physical Sciences and Engineering Chemical Engineering Catalysis
Get Full-Text Now
Don't Miss Today's Special Offer
Price was $35.95
You save - $31
Price after discount Only $4.95
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Full-text PDF Download
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