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A comparative oxidation of cyclohexane catalyzed by N-hydroxyphthalimide and ZSM-5 supported Co(II), Mn(II), Ni(II), Zn(II), Fe(III) with molecular oxygen in the absence of solvents and reductants

Paper ID Volume ID Publish Year Pages File Format Full-Text
51771 46853 2008 4 PDF Available
Title
A comparative oxidation of cyclohexane catalyzed by N-hydroxyphthalimide and ZSM-5 supported Co(II), Mn(II), Ni(II), Zn(II), Fe(III) with molecular oxygen in the absence of solvents and reductants
Abstract

A catalytic system consisting of ZSM-5 supported metal ions (M/ZSM-5) and N-hydroxyphthalimide (NHPI) for the selective oxidation of cyclohexane with dioxygen was reported, and the catalytic activity of various M/ZSM-5 was investigated. Cyclohexane was successfully oxidized in good conversion, the highest conversion of cyclohexane could be obtained using Co(II)/ZSM-5 and NHPI, however, the highest selectivity of adipic acid was from Mn(II)/ZSM-5 and NHPI. The stability and recycling of the catalyst were also reviewed.

Keywords
N-Hydroxyphthalimide; M/ZSM-5; Cyclohexane; Oxidation
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A comparative oxidation of cyclohexane catalyzed by N-hydroxyphthalimide and ZSM-5 supported Co(II), Mn(II), Ni(II), Zn(II), Fe(III) with molecular oxygen in the absence of solvents and reductants
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Publisher
Database: Elsevier - ScienceDirect
Journal: Catalysis Communications - Volume 9, Issue 14, 30 August 2008, Pages 2407–2410
Authors
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Subjects
Physical Sciences and Engineering Chemical Engineering Catalysis
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Price was $35.95
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