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Green catalysis for production of chemicals and CO-free hydrogen

Paper ID Volume ID Publish Year Pages File Format Full-Text
52584 46877 2007 6 PDF Available
Title
Green catalysis for production of chemicals and CO-free hydrogen
Abstract

The precise control of the anchoring mode of molybdenum inside the channels of a ZSM-5 zeolite, i.e. as monomer or dimer, allowed to increase both the activity and the stability of the Mo/ZSM-5 catalyst for the methane dehydro-aromatisation reaction (MDA). By carefully adjusting the reaction conditions, it has been possible to reach for the first time high yields and at the same time avoid deactivation without addition of any oxidant in the flow. Consequently, the MDA reaction can be regarded as an interesting way to convert small methane feedstocks that are usually flared into valuable aromatic compounds and fuel cell grade hydrogen, completely free of CO.

Keywords
Molybdenum; ZSM-5 zeolite; Methane aromatisation; Hydrogen production; Aromatic compounds
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Publisher
Database: Elsevier - ScienceDirect
Journal: Catalysis Communications - Volume 8, Issue 11, November 2007, Pages 1787–1792
Authors
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Subjects
Physical Sciences and Engineering Chemical Engineering Catalysis
Get Full-Text Now
Don't Miss Today's Special Offer
Price was $35.95
You save - $31
Price after discount Only $4.95
100% Money Back Guarantee
Full-text PDF Download
Online Support
Any Questions? feel free to contact us